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Creators/Authors contains: "Kalaj, Mark"

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  1. ; ; ; ; ; (, The Journal of Physical Chemistry C)
    null (Ed.)
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  2. ; ; ; ; ; ; ; (, Chemistry of Materials)
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  3. ; ; ; ; ; ; (, Chemical Reviews)
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  4. ; ; ; ; ; ; (, Chemical Communications)
    Herein, a series of halogenated UiO-66 derivatives was synthesized and analyzed for the breakdown of the chemical warfare agent simulant dimethyl-4-nitrophenyl phosphate (DMNP) to analyze ligand effects. UiO-66-I degrades DMNP at a rate four times faster than the most active previously reported MOFs. MOF defects were quantified and ruled out as a cause for increased activity. Theoretical calculations suggest the enhanced activity of UiO-66-I originates from halogen bonding of the iodine atom to the phosphoester linkage allowing for more rapid hydrolysis of the P–O bond. 
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